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Anthropogenic influences on mercury in Chinese soil and sediment revealed by relationships with total organic carbon
Wen Xue;  Sae Yun Kwon;  Stephan E. Grasby;  Elsie M. Sunderland;  Xin Pan;  Ruiyang Sun;  Ting Zhou;   Haiyu Yan;   Runsheng Yin
2019
Source PublicationEnvironmental Pollution
Volume255Pages:1-8
Abstract

Rapid industrialization has led to high levels of mercury (Hg) releases from anthropogenic sources in China. When deposited to terrestrial ecosystems, Hg has a high affinity for natural organic carbon. This means that Hg concentrations will vary naturally as a function of the total organic carbon (TOC) content of different soils and sediment. Thus, Hg to TOC ratios in topsoil and surface sediment provides a useful normalized tracer of the anthropogenic impact on Hg contamination. We compiled literaturedocumented Hg and total organic carbon (TOC) data for topsoil (n ¼ 957) and surface sediment (n ¼ 1142) in China. Topsoil samples (n ¼ 100) were also collected in this study to broaden the spatial coverage. We found large differences in Hg:TOC ratios among topsoil from background sites, agricultural and urban areas, and mining sites and surface sediment from fluvial, coastal, and marine environments. Specifically, a significant increase in Hg:TOC ratios occurred between soils from background sites (median: Hg:TOC ¼ 21.1; Inter-Quartile Range (IQR): 9.67 to 40.7) and agricultural areas (median: 34.1; IQR: 22.1 to 58.7), urban areas (median: 62.1 ng g1 ; IQR: 34.2 to 154) and mining sites (median: 2780; range: 181 to 43500). Urban and mining sites show the largest increase in Hg:TOC ratios, reflecting elevated anthropogenic Hg inputs in these areas. Fluvial sediment showed higher Hg:TOC ratios (median: 197; IQR: 109 to 389) than coastal (median: 88.3; IQR: 46.8 to 168) and marine sediment (median: 89.7; IQR: 53 to 138), indicating decreased anthropogenic Hg input from rivers to coastal and marine regions. Results of our study suggest Hg:TOC ratios are a useful normalized indicator of the influence of anthropogenic Hg releases on Hg enrichment in topsoil and surface sediment.

KeywordMercury topsoil surface Sediment anthropogenic Influences hg:Toc china
Indexed BySCI
Language英语
Document Type期刊论文
Identifierhttp://ir.gyig.ac.cn/handle/42920512-1/10150
Collection环境地球化学国家重点实验室
Affiliation1.State Key Laboratory of Ore Deposit Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, 550081, Guiyang, China
2.State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, 550081, Guiyang, China
3.University of Chinese Academy of Sciences, 100049, Beijing, China
4.Division of Environmental Science & Engineering, Pohang University of Science and Technology, 77 Cheongam-Ro, Nam Gu, Pohang, 37673, South Korea
5.Geological Survey of Canada, Natural Resources Canada, Calgary, Alberta, T2L 2A7, Canada
6.Harvard John A. Paulson School of Engineering and Applied Sciences, Cambridge, MA, 02138, United States
Recommended Citation
GB/T 7714
Wen Xue;Sae Yun Kwon;Stephan E. Grasby;Elsie M. Sunderland;Xin Pan;Ruiyang Sun;Ting Zhou; Haiyu Yan; Runsheng Yin. Anthropogenic influences on mercury in Chinese soil and sediment revealed by relationships with total organic carbon[J]. Environmental Pollution,2019,255:1-8.
APA Wen Xue;Sae Yun Kwon;Stephan E. Grasby;Elsie M. Sunderland;Xin Pan;Ruiyang Sun;Ting Zhou; Haiyu Yan; Runsheng Yin.(2019).Anthropogenic influences on mercury in Chinese soil and sediment revealed by relationships with total organic carbon.Environmental Pollution,255,1-8.
MLA Wen Xue;Sae Yun Kwon;Stephan E. Grasby;Elsie M. Sunderland;Xin Pan;Ruiyang Sun;Ting Zhou; Haiyu Yan; Runsheng Yin."Anthropogenic influences on mercury in Chinese soil and sediment revealed by relationships with total organic carbon".Environmental Pollution 255(2019):1-8.
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